hmm, you didn't mentioned your MAL(my anime list) so I don't know If you watched them or not but may be try those animes because they are emotional:
Kanon (2006)
Clannad
Fruits Basket
Usagi Drop
Tasogare Otome x Amnesia
Sakurasou no Pet na Kanojo
Golden Time
Cross Game
Kokoro Connect
Little Busters!
3-gatsu no Lion

Ohh and if you can cope with lack of logic in the plot try Symphogear.One of my favorites.(the lack of logic is actualy on purpouse cause it's easier to make emotional scenes).Also it is a music anime and the songs are incredible.

For books: you probably already read it, but- Amber Chronicles from Roger Zelazni (classic in the genre that probably most people know)
Also the The Riftwar Saga from Raymond E. Feist is nice
Another hmm... it's from different genre(sci-fi), but try Vorkosigan Saga from Lois McMaster Bujold. It merge so many things in one - sci-fi, politics,war,romance and many more.

For Light Novels I recomend:
Arifureta Shokugyou de Sekai Saikyou
Mushoku Tensei: Isekai Ittara Honki Dasu
Mahouka Koukou no Rettousei (a lot better than the anime and I love the anime so that says a lot :D )
Tate no Yuusha no Nariagari - realy nice one.I didn't liked just the end, but other than that was great.It's confirmed there will be also an anime.

For Visual Novels- absolutely don't miss Umineko no Naku Koro ni.It changed my life and way of thinking.There is an anime adaptation, but it's weak.It's not containing even 5% of the most epic and phylosophical things.Also when you try it don't forget to tweak (or find already tweaked) version.The original is with amateurish art and without voice acting.The tweaked version is with sprites from the PS3 version nice art.The Voice acting also makes it even better.